Cobaloxime Catalysis: Selective Synthesis of Alkenylphosphine Oxides under Visible Light Wen-Qiang Liu Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, The Chinese Academy of Sciences, Beijing 100190, People’s Republic of China.
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Chloro(pyridine)cobaloxime is a coordination compound containing a Co III center with octahedral coordination. It has been considered as a model compound of vitamin B 12 for studying the properties and mechanism of action of the vitamin.
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The alkene is a central functional group in organic synthesis. While myriad reliable methods exist to access this moiety from other functionalities, acceptorless dehydrogenation, or the direct synthesis of alkenes from alkanes with hydrogen gas as the sole byproduct, remains a challenging, albeit highly desirable, transformation.
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The synthesis of photosensitizers bearing a cobaloxime unit could be sometimes laborious, therefore the design and preparation of new cobaloximes which could be easily introduced in the structure.
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Baran Lab N - H e t e r o c y c l i c C a r b e n e s ( N H C s ) K. J. Eastman 1 An Introduction to N-heterocyclic Carbenes: Prior to 1960, a school of thought that carbenes were too reactive to be isolated thwarted widespread efforts to investigate carbene chemistry.